Highly active, low-cost, and durable electrocatalysts for the water oxidation reaction are pivotal in energy conversion and storage schemes. Here we report the nitride-core, oxide-shell-armor structured FeCoNi oxynitride as an efficient oxygen evolution electrocatalyst with a homogeneously nitride (Fe0.70Co0.56Ni0.92N1.0O0.06) core and oxide (Fe0.4...


NixWO2.72 nanorods (NRs) are synthesized by a one-pot reaction of Ni(acac)2 and WCl4. In the rod structure, Ni(II) intercalates in the defective perovskite-type WO2.72 and is stabilized. The NixWO2.72 NRs show the x-dependent electrocatalysis for the oxygen evolution reaction (OER) in 0.1M KOH with Ni0.78WO2.72 being the most efficient, even outper...
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Hexagonal boron nitride nanosheets (h-BNNs) with rather high specific surface area (SSA) are important two-dimensional layer-structured materials. Here, a solvent-mediated synthesis of h-BNNs revealed a template-free lattice plane control strategy that induced high SSA nanoporous structured h-BNNs with outstanding aerobic oxidative desulfurization...
It’s not hard to see why governments would seek to defend their languages. But some linguists think a staunch anti-English stance may be counterproductive. Truly endangered languages tend to be encroached on mostly by their dominant geographic neighbors, says Selma Sonntag, a political scientist at Humboldt State University who studies language purist movements: “The threat isn’t from English, it’s from whatever the official language is within their area.” Linguist David Crystal, author of “English as a Global Language,” has written about how Welsh-language purism may be furthering an elitism that prevents younger speakers from adopting the tongue. And it’s worth noting that English owes much of its vitality to its long history of borrowing from French, Latin, Arabic, and pretty much any other language it met. “Loanwords...do alter [a language’s] character—but is this a bad thing?” Crystal told me. “Imagine English without French or Latin loanwords. No Shakespeare, for a start.”
Lanthanum-transition-metal perovskites with robust meso-scale porous frameworks (meso-LaMO 3) are synthesized through use of ionic liquids. The resultant samples demonstrate a rather high activity for CO oxidation, by taking advantage of unique nanostructure-derived benefits. This synthesis strategy opens up a new opportunity for preparing functional mesoporous complex oxides of various compositions.
Controlling the physical and chemical properties of alloy nanoparticles (NPs) is an important approach to optimize NP catalysis. Unlike other tuning knobs, such as size, shape and composition, crystal structure has received limited attention and not been well understood for its role in catalysis. This deficiency is mainly due to the difficulty in s...
We report the synthesis of core/shell face-centered tetragonal (fct)-FePd/Pd nanoparticles (NPs) via reductive annealing of core/shell Pd/Fe3O4 NPs followed by temperature-controlled Fe etching in acetic acid. Among three different kinds of core/shell FePd/Pd NPs studied (FePd core at ~8 nm and Pd shell at 0.27, 0.65 or 0.8 nm), the fct-FePd/Pd-0.6...
A simple, solvent-free, solid-state self-assembly strategy for the synthesis of alkaline-metal-oxide-doped mesoporous carbons (MCs) with tunable mesopores (~5-9 nm), high surface-areas (up to 571 m2/g) and large pore volumes (up to 0.65 cm3/g) is developed via the mechanochemical assembly between polyphenol-Ca2+/Mg2+ composites and F127 copolymers....
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